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Occurrence, distribution, and fate evaluation of endocrine disrupting compounds in three wastewater treatment plants with different treatment technologies in Türkiye
Science of The Total Environment 2024 Cilt 952
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Atıf
952
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Özet
Nowadays, two of the endocrine disrupting compounds (EDCs) in the group of alkylphenols (APs), nonylphenol (4-NP) and octylphenol (4-t-OP), have attracted great scientific and regulatory attention mainly due to concerns about their aquatic toxicity and endocrine disrupting activity. This paper investigated the occurrence, distribution behavior, fate, and removal of 4-NP and 4-t-OP in liquid and solid phases of three full-scale wastewater treatment plants (WWTPs) with different treatment technologies comparatively. In this context, (i) advanced biological WWTP, (ii) wastewater stabilization pond (WSP), and (iii) constructed wetland (CW) were utilized. In all three investigated WWTPs, the concentrations of 4-NP (219.9–19,354.4 ng/L) in raw wastewater were higher than those of 4-t-OP (13.9–2822.4 ng/L). Within the scope of annual average removal efficiencies, 4-NP was treated highly in advanced biological WWTP (93.5 %), while it was almost not treated in WSP (3.1 %) and treated with negative removal (<0 %) in CW. While 4-t-OP was treated at a similar removal rate (93.5 %) to 4-NP in advanced biological WWTP, it was treated moderately in WSP (52.5 %) and very poorly in CW (12.4 %). It has been determined that the most important removal mechanism of both 4-NP and 4-t-OP in WWTPs is biodegradation, followed by sorption onto sewage sludge. According to the mass balance performed in advanced biological WWTP, the biodegradation rates for 4-NP and 4-t-OP were found to be 70.4 % and 86.6 %, respectively, while the sorption onto sewage sludge were determined to be 23.3 % and 6.8 %. One of the critical findings obtained within the scope of the study is that while the concentrations of both metabolites, especially 4-NP, in wastewater and sewage sludge, decreased considerably under aerobic conditions, on the contrary, their concentrations increased significantly under anaerobic conditions. Both compounds were detected at higher concentrations in primary sludge compared to secondary sludge in advanced biological WWTP, while in WSP, they were determined at higher concentrations in anaerobic stabilization pond sludge compared to facultative stabilization pond sludge. Besides, it was also determined that the sorption behavior of these alkylphenols is much more dominant than desorption.
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952
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Article
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Kaynak: SCIENCE OF THE TOTAL ENVIRONMENT
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Scimago Dergi Bilgisi Otomatik ISSN Eşleştirmesi 2024 yılı verileri
Science of the Total Environment
Q1
SJR Quartile
2,137
SJR Skoru
399
H-Index
Kategoriler: Environmental Chemistry (Q1) · Environmental Engineering (Q1) · Pollution (Q1) · Waste Management and Disposal (Q1)
Alanlar: Environmental Science
Ülke: Netherlands · Elsevier B.V.
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Anahtar Kelimeler

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Makale Bilgileri

Dergi Science of The Total Environment
ISSN 0048-9697
Yıl 2024 / 11. ay
Cilt / Sayı 952
Makale Türü Özgün Makale
Hakemlik Hakemli
Endeks SCI-Expanded
JCR Quartile Q1
Teşvik Puanı 2,57 · YÖKSİS Akademik Teşvik
Yayın Dili Türkçe
Kapsam Uluslararası
Toplam Yazar 7 kişi
Erişim Türü Basılı+Elektronik
Alan Mühendislik Temel Alanı Biyomühendislik Nanoteknoloji Biyoseparasyon ve Saflaştırma

YÖKSİS Yazar Kaydı

Yazar Adı NAS BİLGEHAN,DOLU TAYLAN,ATEŞ HAVVA,DİNÇ SALİHA,KARA MERYEM,ARGUN MEHMET EMİN,YEL ESRA
YÖKSİS ID 8052764

Metrikler

Scopus Atıf 2
Havuz Atıfları 0
JCR Quartile Q1
Teşvik Puanı 2,57
Yazar Sayısı 7